Interfacial Phenomena in Thin Polymer Films: Phase Coexistence and Segregation

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An Interface Phase Transition: Complete to Partial Wetting

1980 • 290 citations

Emulsifying effects of block copolymers in incompatible polymer blends

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Critical properties of the Flory–Huggins lattice model of polymer mixtures

1987 • 266 citations

A practical guide to polymer miscibility

1990 • 266 citations

Surface Enrichment in an Isotopic Polymer Blend

1989 • 263 citations

Preferential surface adsorption in miscible blends of polystyrene and poly(vinyl methyl ether)

1988 • 261 citations

Observed frustration in confined block copolymers

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Polymer Microscopy

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Model calculations for wetting transitions in polymer mixtures

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Dynamics in spinodal decomposition of polymer mixtures

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Segregation of block copolymers to interfaces between immiscible homopolymers

1990 • 218 citations

Critical Behavior of Binary Liquid Mixtures of Deuterated and Protonated Polymers

1985 • 217 citations

Spinodal decomposition in thin films of a polymer blend

1992 • 206 citations

Thermodynamics and kinetics of grafting end-functionalized polymers to an interface

1990 • 200 citations

Evidence for Capillary Waves at Immiscible Polymer/Polymer Interfaces

1997 • 198 citations

Study of miscibility and critical phenomena of deuterated polystyrene and hydrogenated poly(vinyl methyl ether) by small-angle neutron scattering

1985 • 186 citations

Temperature, composition and molecular-weight dependence of the binary interaction parameter of polystyrene/poly(vinyl methyl ether) blends

1988 • 184 citations

Mean-field theory of polymer interfaces in the presence of block copolymers

1990 • 181 citations

Experimental Observation of Critical Wetting

1996 • 178 citations

Polymer-polymer diffusion in melts

1983 • 178 citations

Novel phase behaviour of a confined fluid or Ising magnet

1992 • 171 citations

Theory of end-adsorbed polymer brushes in polymeric matrices

1991 • 170 citations

Imaging and modification of polymers by scanning tunneling and atomic force microscopy

1988 • 167 citations

Analysis of diffusion in polymers by forward recoil spectrometry

1984 • 165 citations

Integral equation theory of the structure and thermodynamics of polymer blends

1989 • 162 citations

Thermodynamic interactions in model polyolefin blends obtained by small-angle neutron scattering

1992 • 162 citations

Complete Wetting from Polymer Mixtures

1992 • 161 citations

The diffusion of long-chain molecules through bulk polyethelene

1979 • 160 citations

Polymer Interdiffusion

1989 • 157 citations

Isotope-Induced Quantum-Phase Transitions in the Liquid State

1986 • 157 citations

Surface spinodals and extended wetting in fluids and polymer solutions

1983 • 147 citations

Phase Transitions of Polymer Blends and Block Copolymer Melts in Thin Films

1999 • 140 citations

Effects of a diblock copolymer on adhesion between immiscible polymers. 2. Polystyrene (PS)-PMMA copolymer between poly(phenylene oxide) (PPO) and PMMA

1993 • 138 citations

Mean-field and Ising critical behavior of a polymer blend

1987 • 136 citations

A lattice model for the surface segregation of polymer chains due to molecular weight effects

1990 • 134 citations

Structural Origin of Thermodynamic Interactions in Blends of Saturated Hydrocarbon Polymers

1994 • 134 citations

Regular and Irregular Mixing in Blends of Saturated Hydrocarbon Polymers

1995 • 133 citations

Anomalous size-dependence of interfacial profiles between coexisting phases of polymer mixtures in thin-film geometry: A Monte Carlo simulation

1997 • 130 citations

Soft Order in Physical Systems

1994 • 127 citations

Effect of monomer structure and compressibility on the properties of multicomponent polymer blends and solutions. 3. Application to deuterated polystyrene [PS(D)]poly(vinyl methyl ether) (PVME) blends

1991 • 127 citations

Interference of spinodal waves in thin polymer films

1993 • 124 citations

Theory of diblock-copolymer segregation to the interface and free surface of a homopolymer layer

1992 • 124 citations

Ordering in Macromolecular Systems

1994 • 123 citations

Real space observation of dynamic scaling in a critical polymer mixture

1993 • 122 citations

Advances in Polymer Science

1992 • 122 citations

Wetting Transition in Lutidine-Water Mixtures

1982 • 118 citations

First-order wetting transition at a liquid–vapor interface

1983 • 114 citations

The Form of the Enriched Surface Layer in Polymer Blends

1990 • 114 citations

Composition Dependence of the Interaction Parameter in Isotopic Polymer Blends

1994 • 113 citations

Influence of surface interactions on spinodal decomposition

1993 • 110 citations

Grafted polymer brushes in polymeric matrices

1996 • 109 citations

Reversal of the isotopic effect in the surface behavior of binary polymer blends

1993 • 108 citations

The Interdiffusion of Polymers

1990 • 108 citations

Thermodynamics of Mixing for Blends of Model Ethylene-Butene Copolymers

1994 • 106 citations

Thermodynamics of isotopic polymer mixtures: Significance of local structural symmetry

1988 • 104 citations

End-Tethered Chains in Polymeric Matrixes

1995 • 103 citations

Thermodynamics of isotopic polymer mixtures: poly(vinylethylene) and poly(ethylethylene)

1988 • 103 citations

Diffusion-Limited Growth of Wetting Layers

1986 • 103 citations

Interfacial segregation in two-phase polymer blends with diblock copolymer additives: the effect of homopolymer molecular weight

1992 • 102 citations

Surface segregation in binary polymer mixtures: a lattice model

1991 • 102 citations

Segregation of block copolymer micelles to surfaces and interfaces

1991 • 100 citations

Dynamics of surface enrichment: A theory based on the Kawasaki spin-exchange model in the presence of a wall

1991 • 100 citations

Entropy-driven surface segregation in block copolymer melts

1993 • 98 citations

Effect of deuterium substitution on thermodynamic interactions in polymer blends

1993 • 97 citations

Creation of Stable Poly(ethylene oxide) Surfaces on Poly(methyl methacrylate) Using Blends of Branched and Linear Polymers

1997 • 96 citations

Interfacial phase transitions in block copolymer/homopolymer blends

1993 • 95 citations

Determining the temperature-dependent Flory interaction parameter for strongly immiscible polymers from block copolymer segregation measurements

1994 • 95 citations

Entangled polymers

1983 • 94 citations

The surface composition of miscible polymer blends

1993 • 93 citations

Critical Fluctuations in a Binary Polymer Mixture

1983 • 93 citations

Segment density distribution of symmetric diblock copolymers at the interface between two homopolymers as revealed by neutron reflectivity

1991 • 89 citations

Structure at polymer interfaces determined by high-resolution nuclear reaction analysis

1990 • 89 citations

Evidence for Size Effects on Interfacial Widths in Confined Thin Films

1996 • 89 citations

Studies of surface and interface segregation in polymer blends by secondary ion mass spectrometry

1992 • 88 citations

Determination of the concentration profile at the surface of deuterated polystyrene/hydrogenated polystyrene blends using high-resolution ion scattering techniques

1991 • 88 citations

Interfacial segment density profiles of end-anchored polymers in a melt

1992 • 88 citations

Molecular weight scaling in critical polymer mixtures

1992 • 87 citations

Non-ideal mixing in binary blends of perdeuterated and protonated polystyrenes

1986 • 83 citations

Relationships between polymer interaction parameters

1989 • 82 citations

Surface phase inversion in finite-sized binary mixtures

1994 • 82 citations

Self-assembly of a homopolymer mixture via phase separation

1994 • 80 citations

Bulk and Interface Thermodynamics of Polymer Alloys

1983 • 79 citations

Interfacial studies of incompressible binary blends

1991 • 78 citations

Effect of bimodal molecular weight distribution on the polymer brush

1993 • 76 citations

The compositional dependence of thermodynamic interactions in blends of model polyolefins

1994 • 76 citations

Effect of Architecture in the Surface Segregation of Polymer Blends

1996 • 75 citations

Surface effects on polymer blends and block copolymer melts: Theoretical concepts of surface enrichment, surface induced phase separation and ordering

1995 • 75 citations

Critical fluctuations and relaxation phenomena in the isotopic blend polystyrene/deuteropolystyrene investigated by small angle neutron scattering

1990 • 74 citations

Wetting of Substrates with Phase-Separated Binary Polymer Mixtures

1997 • 74 citations

Early state of spinodal decomposition studied with small angle neutron scattering in the blend deuteropolystyrene and polyvinylmethylether: A comparison with the Cahn–Hilliard–Cook theory

1992 • 74 citations

Use of the D(3He,P)4 He reaction to study polymer diffusion in polymer melts

1989 • 73 citations

Surface segregation in polymer blends due to stiffness disparity

1994 • 73 citations

Entropic and Enthalpic Surface Segregation from Blends of Branched and Linear Polymers

1995 • 70 citations

Theory of a planar grafted chain layer immersed in a solution of mobile polymer

1991 • 70 citations

Transient Wetting and 2D Spinodal Decomposition in a Binary Polymer Blend

1995 • 69 citations

Influence of blend compressibility on extrapolated zero-angle coherent scattering and spinodal: limitations of RPA [random-phase approximation] analysis

1990 • 69 citations

Surface directed spinodal decomposition in a partially miscible polymer blend

1995 • 68 citations

Nucleation and growth of monodisperse droplets in a binary-fluid system

1990 • 68 citations

SAXS study of micelle formation in mixtures of butadiene homopolymer and styrene-butadiene block copolymer. 3. Comparison with theory

1986 • 67 citations

Interfacial structure in polymer mixtures below the critical point

1989 • 67 citations

Miscibility and phase separation in poly(methyl methacrylate)/poly(vinyl chloride) blends: study of thermodynamics by thermal analysis

1992 • 66 citations

Structure of a bidisperse polymer brush: Monte Carlo simulation and self-consistent field results

1992 • 65 citations

Investigation of diffusion in polystyrene using secondary ion mass spectroscopy

1989 • 65 citations

Microstructure and isotopic labeling effects on the miscibility of polybutadiene blends studied by the small-angle neutron scattering technique

1990 • 64 citations

Small-angle neutron scattering by partially deuterated polymers and their blends

1994 • 64 citations

Quasielastic Scattering by Semidilute Polymer Solutions

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The effect of finite film thickness on the surface segregation in symmetric binary polymer mixtures

1993 • 61 citations

Vanishing interfacial tension in an immiscible polymer blend

1992 • 59 citations

Structure-Property Correlations of Atomistic and Coarse-Grained Models of Polymer Melts

1995 • 59 citations

Deuteration Effects and Solubility Parameter Ordering in Blends of Saturated Hydrocarbon Polymers

1994 • 58 citations

Lattice theory of polymer blends and liquid mixtures: Beyond the Flory–Huggins approximation

1989 • 56 citations

Thermodynamics and phase separation in melt blends of polyethylene and model copolymers

1991 • 56 citations

The Structure of Grafted Polystyrene Layers in a Range of Matrix Polymers

1995 • 54 citations

Surface phase behavior in binary polymer mixtures. I. Miscibility, phase coexistence, and interactions in polyolefin blends

1996 • 53 citations

Reflection-scanning near-field optical microscopy and spectroscopy of opaque samples

1994 • 52 citations

On the N-scaling of the Ginzburg number and the critical amplitudes in various compatible polymer blends

1994 • 52 citations

Block copolymers at interfaces. 2. Surface adsorption

1988 • 52 citations

Segregation of low molecular weight symmetric diblock copolymers at the interface of high molecular weight homopolymers

1991 • 51 citations

Influence of broken conformational symmetry on the surface enrichment of polymer blends

1992 • 51 citations

Enthalpy-driven swelling of a polymer brush

1990 • 50 citations

Brush formation from mixtures of short and long end-functionalized chains in a good solvent

1993 • 50 citations

Depth profiling methods that provide information complementary to neutron reflectivity

1991 • 49 citations

Critical wetting in two-component polymer blends

1989 • 49 citations

Adsorption of Semiflexible Polymers

1996 • 48 citations

Kinetics of formation of a surface enriched layer in an isotopic polymer blend

1990 • 48 citations

Surface segregation in conformationally asymmetric polymer blends: Incompressibility and boundary conditions

1996 • 48 citations

Phase separation of symmetrical polymer mixtures in thin-film geometry

1995 • 48 citations

Effect of long-range surface interactions on wetting transitions of polymer mixtures

1991 • 47 citations

Influence of chain length on the interface width of an incompatible polymer blend

1996 • 47 citations

The effects of confinement and surface interactions on coexistence in a binary polymer mixture

1992 • 47 citations

Surface phase behavior in binary polymer mixtures. II. Surface enrichment from polyolefin blends

1996 • 47 citations

Behavior of isotopic, binary polymer blends in the vicinity of neutral surfaces: the effects of chain-length disparity

1991 • 43 citations

Relationship among polymer-polymer interaction energy densities and the deuterium isotope effect

1987 • 42 citations

Neutron Reflectometry Study of Surface Segregation in an Isotopic Poly(ethylenepropylene) Blend: Deviation from Mean-Field Theory

1995 • 42 citations

Wetting transitions in polymer blends: A Monte Carlo lattice simulation

1991 • 42 citations

Equilibrium Segment Density Distribution of a Diblock Copolymer Segregated to the Polymer/Polymer Interface

1994 • 42 citations

Configuration of grafted polystyrene chains in the melt: Temperature and concentration dependence

1992 • 40 citations

Surface Enrichment in a Miscible Polymer Blend: An Experimental Test of Self-Consistent Field and Long-Wavelength Approximation Models

1996 • 40 citations

Evidence Against the Integral Equation Theory of Polymer Blends

1992 • 40 citations

Thermodynamics of polyolefin blends: small-angle neutron scattering studies with partially deuterated chains

1990 • 40 citations

First-order wetting transitions of polymer mixtures in contact with a wall

1989 • 39 citations

Isotope and microstructure interactions in blends of random copolymers

1993 • 38 citations

Effect of long-range forces on surface enrichment in polymer blends

1993 • 37 citations

Measuring the binodal by interdiffusion in blends of deuterated polystyrene and poly(styrene-co-4-bromostyrene)

1991 • 37 citations

Improved hydrogen and deuterium depth profiling in polymers using low energy forward recoil spectrometry

1994 • 37 citations

Dynamics of mixing between partially miscible polymers

1990 • 37 citations

Design of miscible polyolefin copolymer blends

1995 • 36 citations

Growth of Wetting Layers from Liquid Mixtures

1996 • 36 citations

Phase transitions in thin films of symmetric binary polymer mixtures

1994 • 36 citations

Effect of Brush Polydispersity on the Interphase between End-Grafted Brushes and Polymeric Matrixes

1994 • 35 citations

Theory for the chi parameter of polymer blends: Effect of attractive interactions

1988 • 35 citations

Interfacial Aspects of Multicomponent Polymer Materials

1997 • 35 citations

Thermal concentration fluctuations of block polymer/homopolymer mixtures in the disordered state. 1. Binary mixtures of SI/HS

1991 • 35 citations

Surface-Directed Spinodal Decomposition in the Blend of Polystyrene and Tetramethyl-Bisphenol-A Polycarbonate

1994 • 34 citations

Strongly stretched polymer brushes

1994 • 33 citations

Segregation Study of a BAB Triblock Copolymer at the A/B Homopolymer Interface

1994 • 32 citations

The effects of local stiffness disparity on the surface segregation from binary polymer blends

1995 • 32 citations

Liquid‐liquid phase separation in multicomponent polymer systems, 21. Deuterium isotope effect in polymer compatibility

1984 • 31 citations

Kinetics of formation of physically end-adsorbed polystyrene layers from the melt

1994 • 31 citations

Critical temperature shifts in thin polymer blend films

1994 • 31 citations

Concentration profile near the surface of polymer mixtures: a Monte Carlo study

1996 • 31 citations

Palaeotemperatures from tree rings and the D/H ratio of cellulose as a biochemical thermometer

1975 • 31 citations

Coexistence in a Binary Isotopic Polymer Mixture

1992 • 31 citations

Light‐scattering studies on phase separation in a binary blend with addition of diblock copolymers

1995 • 30 citations

Adsorption of copolymer chains from a melt onto a flat surface

1992 • 29 citations

Self‐diffusion in melts of statistical copolymers: The effect of changes in microstructural composition

1995 • 29 citations

Tailored Polymer Surfaces

1997 • 28 citations

Technique for the study of diffusion of large molecules in polymers based on infrared microdensitometry

1975 • 28 citations

Surface Segregation in Diblock Copolymers and Polymer Blend Thin Films

1995 • 28 citations

Phase coexistence in binary mixtures in thin films with symmetric walls: model calculations for two- and three-dimensional Ising lattices

1997 • 27 citations

Interdiffusion in binary polymer mixtures

1993 • 27 citations

Miscibility of poly (styrene‐co‐methylmethacrylate)s differing in composition

1990 • 27 citations

Order-Induced Period Doubling during Surface-Directed Spinodal Decomposition

1994 • 27 citations

Brush Formation by Symmetric and by Highly Asymmetric Diblock Copolymers at Homopolymer Interfaces

1995 • 26 citations

The wetting transition for polymer mixtures

1994 • 26 citations

Miscibility in blends of model polyolefins and corresponding diblock copolymers: thermal analysis studies

1993 • 26 citations

Matrix-Modulated Swelling of a Polymer Brush

1992 • 26 citations

Phase Separation Versus Wetting: a Mean Field Theory for Symmetrical Polymer Mixtures Confined Between Selectively Attractive Walls

1996 • 25 citations

Interfacial behavior of compressible polymer blends

1993 • 25 citations

Berechnung von Mischungswärmen kondensierter Systeme

1925 • 25 citations

Surface segregation in a polymer blend. Comparison between Monte Carlo simulation and mean-field theory

1993 • 24 citations

Neutron Scattering Studies of Surfaces and Interfaces

1990 • 24 citations

Phenomenological theory for the formation of interfaces via the interdiffusion of layers

1991 • 23 citations

Conformation of Grafted Polystyrene Chains in a Melt

1991 • 23 citations

Interdiffusion in the partially miscible polymer blend of deuterated polystyrene and poly(styrene-co-bromostyrene)

1989 • 22 citations

Phase transitions in thin films of a binary mixture

1992 • 22 citations

Compressibility Effects in the Analysis and Interpretation of Neutron Scattering Data from Polymer Blends

1996 • 22 citations

Diblock copolymers attached to homopolymer surfaces and interfaces

1993 • 21 citations

Surface segregation amplification in miscible polymer blends near criticality

1997 • 21 citations

On the Control of Surface Enrichment in Polymer Blends and Copolymers

1997 • 21 citations

Toward a Molecular Basis for Understanding the Behavior of Isotopic Polymer Blends: Lattice Cluster Theory Computations for PSD/PSH Blends

1994 • 21 citations

Segregation at the Interface between a Homopolymer and a Binary Polymer Blend

1995 • 20 citations

Surface-tethered polymers in polymeric matrices

1993 • 20 citations

Surface Phase Transition in a Polymer Blend

1993 • 20 citations

Molecular weight dependence of diblock copolymer segregation at a polymer/polymer interface

1994 • 19 citations

Critical point wetting from binary polymer mixtures

1994 • 19 citations

Surface phase behavior in binary polymer mixtures. III. Temperature dependence of surface enrichment and of wetting

1997 • 19 citations

Miscibility behavior in blends of poly(acrylonitrile-co-butadiene) and chlorinated poly(vinyl chloride)

1992 • 18 citations

Modification of long-ranged forces by surface exchange of polymeric amphiphiles

1992 • 18 citations

Influence of conformational asymmetry on the surface enrichment of polymer blends II

1995 • 17 citations

Nematic–smectic-Cphase transition in the polymeric liquid crystalC-6 polysiloxane: A high resolution x-ray study

1987 • 17 citations

Near-Surface Composition Profiles in Isotopic Polymer Blends Determined via High-Resolution Nuclear Reaction Analysis

1998 • 17 citations

Kinetics of interface formation between weakly incompatible polymer blends

1990 • 17 citations

Real‐space composition–depth profiling in polymeric samples to 3 nm resolution using the ²H(³He, ¹H)⁴He nuclear reaction

1997 • 16 citations

Concentration Profiles of End-Grafted, Diblock and Triblock Polymers in the Melt: Near-Wall Structure and Effects of Segment-Wall Interaction

1995 • 15 citations

Surface-directed spinodal decomposition modified by a surface active copolymer

1997 • 15 citations

Surface enrichment in blends of miscible polymers

1994 • 15 citations

Interference of microstructure and isotope labeling effects in polymer blend compatibility

1993 • 15 citations

Diffusion‐Limited Segregation of Diblock Copolymers to a Homopolymer Surface

1995 • 13 citations

Segment density profiles of end-adsorbed polymers in chemically identical melts

1994 • 12 citations

The free energy of a binary mixture near a surface with applications to surface enrichment

1992 • 11 citations

Neutron reflectivity of end grafted polymers in poor solvent: Kinetic effects

1996 • 9 citations

Surface enrichment-depletion duality in a binary polymer blend

1998 • 8 citations

Hyperbolic tangent variational approximation for interfacial profiles of binary polymer blends

1995 • 8 citations

The Enrichment-Depletion Duality as an Indicator of Critical Wetting in Polymer Blends

1994 • 8 citations

Competitive Adsorption at Homopolymer Interfaces from a Binary Mixture of Diblock Copolymers

1995 • 7 citations

A self-consistent field study of the wetting transition in binary polymer blends

1997 • 6 citations

Polymers and thermodynamics

1987 • 6 citations

Thin films of a binary polymer mixture: calculations of the concentration profile for asymmetric walls

1996 • 5 citations

Effect of deuterium substitution on the surface interactions in binary polymer mixtures

1998 • 5 citations

Untitled

1998 • 2 citations

Deleted Work

1955 • 0 citations